基于铅稳定同位素的多金属复合污染土壤源解析新思路——以西南地区某矿区农田为例
作者:
作者单位:

作者简介:

通讯作者:

中图分类号:

X53

基金项目:

国家自然科学基金项目(42077118)和国家重点研发计划项目(2020YFC1808000)资助。


Fresh Insights into Source Identification of Multi-elements in Soil with Stable Pb Isotope: A Case Study of Mining-affected Agricultural Land
Author:
Affiliation:

Fund Project:

National Natural Science Foundation of China (Grant No. 42077118), and National Key Research and Development Program of China (Grant No. 2020YFC1808000)

  • 摘要
  • |
  • 图/表
  • |
  • 访问统计
  • |
  • 参考文献
  • |
  • 相似文献
  • |
  • 引证文献
  • |
  • 资源附件
  • |
  • 文章评论
    摘要:

    本文以我国西南某矿区典型多金属复合污染农田土壤为例,基于铅(Pb)稳定同位素分析,结合矿物学分析,对土壤Pb来源进行定量解析,并针对其他重金属来源进行外推。同位素源解析结果表明,人为源对于土壤重金属的贡献率高达61%~89%,矿渣浸沥与矿区道路扬尘为主要的污染途径。矿物学分析能够辅助印证Pb稳定同位素分析结果,在一定程度上克服由于污染源信号重叠造成的源解析困难。通过相关分析,可以将Pb同位素源解析的结果合理外推,在一定程度上解释其他重金属元素的来源。本文提出的源解析新思路能够高效、准确地解析多金属复合污染土壤中重金属元素的来源,尤其适用于我国土壤多金属复合污染集中连片存在、成因复杂的现状,具有很强的现实意义。

    Abstract:

    In this study, an integrated approach for the source identification of multi-elements in soil was proposed. Stable Pb isotopes, with the help of mineralogical approaches, have successfully been applied for the source identification of a multi-metal contaminated agricultural soil in a typical mining district in Southwest China. Quantitative analysis of source contributions revealed that the anthropogenic sources accounted for 61%-89% of soil metal accumulation. Stable isotope analysis indicated that mining waste leaching and mining dust raising from the road both contribute to soil contamination, but the signals of these two processes were overlapped, making it impossible to distinguish the contribution of each. Mineralogical analysis has therefore been used to aid in source identification. Considering that concentrations of other metals correlate well with Pb, it is suggested that the results from Pb isotope analysis could be further extrapolated to reveal the sources of other soil metals.

    参考文献
    相似文献
    引证文献
引用本文

王刘炜,程敏,邓渠成,侯仁杰,侯德义.基于铅稳定同位素的多金属复合污染土壤源解析新思路——以西南地区某矿区农田为例[J].土壤,2022,54(5):1032-1040. WANG Liuwei, CHENG Min, DENG Qucheng, HOU Renjie, HOU Deyi. Fresh Insights into Source Identification of Multi-elements in Soil with Stable Pb Isotope: A Case Study of Mining-affected Agricultural Land[J]. Soils,2022,54(5):1032-1040

复制
分享
文章指标
  • 点击次数:
  • 下载次数:
  • HTML阅读次数:
  • 引用次数:
历史
  • 收稿日期:2022-01-28
  • 最后修改日期:2022-03-24
  • 录用日期:2022-03-29
  • 在线发布日期: 2022-10-31
  • 出版日期: