To alleviate aluminum (Al) toxicity to the normal growth and efficient metal removal by hyperaccumulators in acid soils, the efficiencies of different strategies to relieve Al stress on cadmium (Cd) hyperaccumulator Sedum plumbizincicola were compared. The results show that in the hydroponic experiment, Zn addition significantly enhances root Cd²⁺ uptake rate by S.plumbizincicola under Al stress while adding CaCl₂ or citric acid to solution has no significant effect on root Cd²⁺ uptake. In the pot experiment, adding lime significantly increases soil pH, and enhances the growth and shoot Cd uptake of the hyperaccumulating plant. However, adding rice or maize biochars, or citric acid in soil does not significantly alleviate the inhibition of plant growth and Cd uptake raised by Al stress. In contrast, adding citric acid aggravates soil acidification. Agricultural strategy of intercropping with S.plumbizincicola and buckwheat was also used to alleviate Al stress, which decreases soil Al activity to some extent and does not significantly affect shoot Cd uptake per plant by S.plumbizincicola with appropriate planting density. Above all, using a combined strategy of intercropping with the hyperaccumulator and Al-tolerant crop with the application of soil amendment to alleviate Al toxicity will not significantly decrease soil Cd availability and plant Cd uptake, thus can realize remediation and crop production simultaneously in Al-stressed soils.